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Journal Articles

Evaluation of the remaining spent extraction solvent in vermiculite after leaching tests via PIXE analysis

Arai, Yoichi; Watanabe, So; Hasegawa, Kenta; Okamura, Nobuo; Watanabe, Masayuki; Takeda, Keisuke*; Fukumoto, Hiroki*; Ago, Tomohiro*; Hagura, Naoto*; Tsukahara, Takehiko*

Nuclear Instruments and Methods in Physics Research B, 542, p.206 - 213, 2023/09

 Times Cited Count:0 Percentile:0.02(Instruments & Instrumentation)

Journal Articles

Improvement in the elution performance of an N,N,N',N-tetraoctyl diglycolamide impregnated extraction chromatography adsorbent using neodymium via micro-particle-induced X-ray emission analysis

Takahatake, Yoko; Watanabe, So; Arai, Tsuyoshi*; Sato, Takahiro*; Shibata, Atsuhiro

Applied Radiation and Isotopes, 196, p.110783_1 - 110783_5, 2023/06

 Times Cited Count:0 Percentile:0.01(Chemistry, Inorganic & Nuclear)

Journal Articles

Actual stress analysis of small-bore butt-welded pipe by complementary use of synchrotron X-rays and neutrons

Suzuki, Kenji*; Miura, Yasufumi*; Shiro, Ayumi*; Toyokawa, Hidenori*; Saji, Choji*; Shobu, Takahisa; Morooka, Satoshi

Zairyo, 72(4), p.316 - 323, 2023/04

Journal Articles

Development of the multi-cubic $$gamma$$-ray spectrometer and its performance under intense $$^{137}$$Cs and $$^{60}$$Co radiation fields

Kaburagi, Masaaki; Shimazoe, Kenji*; Kato, Masahiro*; Kurosawa, Tadahiro*; Kamada, Kei*; Kim, K. J.*; Yoshino, Masao*; Shoji, Yasuhiro*; Yoshikawa, Akira*; Takahashi, Hiroyuki*

Nuclear Instruments and Methods in Physics Research A, 1010, p.165544_1 - 165544_9, 2021/09

 Times Cited Count:0 Percentile:0.02(Instruments & Instrumentation)

The number of nuclear facilities being decommissioned has been increasing worldwide, in particular following the accident of the Tokyo Electric Power Company Holdings' Fukushima Daiichi Nuclear Power Station in 2011. In these nuclear facilities, proper management of radioactive materials is required. Then, A $$gamma$$-ray spectrometer with four segmentations using small volume CeBr$$_{3}$$ scintillators with a dimension of $$5 times 5 times 5$$ $$rm{mm}^3$$ was developed. The four scintillators were coupled to a multi-anode photomultiplier tube specific to intense radiation fields. We performed the $$gamma$$-ray exposure study under $$^{137}$$Cs and $$^{60}$$Co radiation fields. Under the $$^{137}$$Cs radiation field, the relative energy resolution at 1375 mSv/h was the relative energy resolution at 1375 mSv/h was 9.2$$pm$$0.05%, 8.0$$pm$$0.08%, 8.0$$pm$$0.03%, and 9.0$$pm$$0.04% for the four channels, respectively.

Journal Articles

Microscopic analyses on Zr adsorbed IDA chelating resin by PIXE and EXAFS

Arai, Yoichi; Watanabe, So; Ono, Shimpei; Nomura, Kazunori; Nakamura, Fumiya*; Arai, Tsuyoshi*; Seko, Noriaki*; Hoshina, Hiroyuki*; Hagura, Naoto*; Kubota, Toshio*

Nuclear Instruments and Methods in Physics Research B, 477, p.54 - 59, 2020/08

 Times Cited Count:5 Percentile:45.45(Instruments & Instrumentation)

Journal Articles

Quantitative analysis of Zr adsorbed on IDA chelating resin using Micro-PIXE

Arai, Yoichi; Watanabe, So; Ono, Shimpei; Nomura, Kazunori; Nakamura, Fumiya*; Arai, Tsuyoshi*; Seko, Noriaki*; Hoshina, Hiroyuki*; Kubota, Toshio*

QST-M-23; QST Takasaki Annual Report 2018, P. 59, 2020/03

Journal Articles

Micro-PIXE analysis study of ferrite products synthesized from simulated radioactive liquid waste containing chemical hazardous elements

Abe, Tomohisa; Shimazaki, Takejiro; Osugi, Takeshi; Nakazawa, Osamu; Yamada, Naoto*; Yuri, Yosuke*; Sato, Takahiro*

QST-M-16; QST Takasaki Annual Report 2017, P. 140, 2019/03

no abstracts in English

Journal Articles

Application of ferrite process to radioactive waste; Study of ferrite product stability by micro-PIXE analysis

Abe, Tomohisa; Shimazaki, Takejiro; Osugi, Takeshi; Yamada, Naoto*; Yuri, Yosuke*; Sato, Takahiro*

QST-M-8; QST Takasaki Annual Report 2016, P. 61, 2018/03

no abstracts in English

Journal Articles

Micro-PIXE analysis on adsorbent of extraction chromatography for MA(III) recovery

Takahatake, Yoko; Watanabe, So; Kofuji, Hirohide; Takeuchi, Masayuki; Nomura, Kazunori; Sato, Takahiro*

International Journal of PIXE, 26(3&4), p.73 - 83, 2017/09

BB2016-1248.pdf:0.36MB

JAEA has been conducting research and development of MA(III) recovery from HLLW by extraction chromatography technology for reduction in amount and environmental impact of radioactive waste. The behavior of adsorbed cations inside the adsorbent packed in a column is necessary to be evaluated for improvement of the adsorbent or flow-sheet to achieve targeted MA(III) recovery performance. In this paper, micro-PIXE analysis was carried out on the particles sampled from various positions of the column to reveal the behavior of cations inside the packed column with CMPO/SiO $$_{2}$$-P adsorbent. Simple experiment and data analysis were shown to be effective to reveal inside of the column, and formation and transportation of the adsorption bands were observed for some cations which are extractable by the CMPO extractant. Some part of Zr(IV) and Mo(VI) were found to remain inside the column without distinct transportation even after the elution operation.

Journal Articles

Local structure and distribution of remaining elements inside extraction chromatography adsorbents

Watanabe, So; Sano, Yuichi; Shiwaku, Hideaki; Yaita, Tsuyoshi; Ono, Shimpei*; Arai, Tsuyoshi*; Matsuura, Haruaki*; Koka, Masashi*; Sato, Takahiro*

Nuclear Instruments and Methods in Physics Research B, 404, p.202 - 206, 2017/08

 Times Cited Count:3 Percentile:28.82(Instruments & Instrumentation)

Journal Articles

Microscopic analyses of complexes formed in adsorbent for Mo and Zr separation chromatography

Abe, Ryoji*; Nagoshi, Kohei*; Arai, Tsuyoshi*; Watanabe, So; Sano, Yuichi; Matsuura, Haruaki*; Takagi, Hideaki*; Shimizu, Nobutaka*; Koka, Masashi*; Sato, Takahiro*

Nuclear Instruments and Methods in Physics Research B, 404, p.173 - 178, 2017/08

 Times Cited Count:5 Percentile:44.54(Instruments & Instrumentation)

Journal Articles

Particle induced X-ray emission-computed tomography analysis of an adsorbent for extraction chromatography

Sato, Takahiro; Yokoyama, Akihito; Kitamura, Akane; Okubo, Takeru; Ishii, Yasuyuki; Takahatake, Yoko; Watanabe, So; Koma, Yoshikazu; Kada, Wataru*

Nuclear Instruments and Methods in Physics Research B, 371, p.419 - 423, 2016/03

 Times Cited Count:7 Percentile:55.03(Instruments & Instrumentation)

Journal Articles

Correction of X-ray detection yield in micro-PIXE analysis according to sample thickness variation measured by STIM

Sato, Takahiro; Sakai, Takuro; Oikawa, Masakazu*

Nuclear Instruments and Methods in Physics Research B, 249(1-2), p.234 - 237, 2006/08

 Times Cited Count:7 Percentile:47.51(Instruments & Instrumentation)

The purpose of this study is to correct yields of characteristic X-ray in micro-PIXE analysis by using STIM and computer simulation. To compensate the reduction of X-ray yields, thickness and internal constitution of a sample must be taken accurately with spatial resolution of a few microns. Therefore, we use STIM to investigate them. Furthermore, we developed a computer software code to correct the X-ray yields. To confirm validity of our method, ion exchange resins, which are similar to biological cells in size, were used as a test sample. There were some wrong distributions of sodium in micro-PIXE analysis of ion exchange resins. But, they could be corrected to some extent by using our code.

Journal Articles

Structural analysis of (Ga,Mn)N epilayers and self-organized dots using MeV ion channeling

Kuroda, Shinji*; Marcet, S.*; Bellet-Amalric, E.*; Cibert, J.*; Mariette, H.*; Yamamoto, Shunya; Sakai, Takuro; Oshima, Takeshi; Ito, Hisayoshi

Physica Status Solidi (A), 203(7), p.1724 - 1728, 2006/05

 Times Cited Count:6 Percentile:31.23(Materials Science, Multidisciplinary)

no abstracts in English

Journal Articles

Measurement of thickness of samples by STIM for PIXE analysis

Sato, Takahiro; Sakai, Takuro; Oikawa, Masakazu*

JAEA-Review 2005-001, TIARA Annual Report 2004, p.304 - 306, 2006/01

The purpose of this study is to correct yields of characteristic X-ray in micro-PIXE analysis by using STIM and computer simulation. To compensate the reduction of X-ray yields, thickness of a sample must be taken accurately with spatial resolution of a few microns but it is difficult to measure them by micro-PIXE analysis. Therefore, we use STIM to investigate them. Furthermore, we developed a computer simulation code to correct the X-ray yields. To confirm validity of our code, ion exchange resins, which are similar to biological cells in size, were used as a test sample. There were some wrong distributions of sodium in micro-PIXE analysis of ion exchange resins. But, they could be corrected to some extent by using our code.

Journal Articles

Micro-PIXE for the study of atmospheric environment

Kasahara, Mikio*; Ma, C.-J.*; Okumura, Motonori*; Kojima, Takuji; Hakoda, Teruyuki; Taguchi, Mitsumasa; Sakai, Takuro; Ohara, Yoshihiro

JAEA-Review 2005-001, TIARA Annual Report 2004, p.293 - 295, 2006/01

Artificial cloud generation experiment was performed using a huge vertical pit located in Kamaishi iron-copper mine to investigate the characteristics of cloud. The physical and chemical properties of individual cloud droplets were examined by microscopic analysis at Kyoto university and micro-PIXE analysis at TIARA. The process of growth of cloud was clarified based on the result on droplet size, its distribution, droplet number concentration, and the change in distribution of chlorine in droplet as the function of size.

Journal Articles

Measurement of thickness of samples by STIM for PIXE analysis

Sato, Takahiro; Sakai, Takuro; Oikawa, Masakazu*

JAEA-Review 2005-001, TIARA Annual Report 2004, p.304 - 306, 2006/01

The purpose of this study is to correct yields of characteristic X-ray in micro-PIXE analysis by using STIM and computer simulation. To compensate the reduction of X-ray yields, thickness of a sample must be taken accurately with spatial resolution of a few microns but it is difficult to measure them by micro-PIXE analysis. Therefore, we use STIM to investigate them. Furthermore, we developed a computer simulation code to correct the X-ray yields. To confirm validity of our code, ion exchange resins, which are similar to biological cells in size, were used as a test sample. There were some wrong distributions of sodium in micro-PIXE analysis of ion exchange resins. But, they could be corrected to some extent by using our code.

Journal Articles

A Report on TIARA Research Review Meeting

Arakawa, Kazuo

Hoshasen Kagaku, (80), p.57 - 59, 2005/09

no abstracts in English

Journal Articles

Application of micro-PIXE to quantitative analysis of heavy elements sorbed on minerals

Kozai, Naofumi; Mitamura, Hisayoshi; Onuki, Toshihiko; Sakai, Takuro; Sato, Takahiro; Oikawa, Masakazu*

Nuclear Instruments and Methods in Physics Research B, 231(1-4), p.530 - 535, 2005/04

 Times Cited Count:9 Percentile:55.97(Instruments & Instrumentation)

Applicability of micro-PIXE analysis to quantitative evaluation of heavy elements sorbed on minerals was investigated to get better understanding of sorption and distribution of heavy elements onto mixture of minerals in soil. For this, external standards, that is, heavy element-sorbing minerals of uniform shape and size, were analyzed by micro-PIXE. It was found that such external standards were available to quantitative evaluation by micro-PIXE though their applicability may be limited.

Journal Articles

Mechanisms of arsenic immobilization in a biomat from mine discharge water

Onuki, Toshihiko; Sakamoto, Fuminori; Kozai, Naofumi; Ozaki, Takuo; Yoshida, Takahiro; Narumi, Issei; Wakai, Eiichi; Sakai, Takuro; Francis, A. J.*

Chemical Geology, 212(3-4), p.279 - 290, 2004/12

 Times Cited Count:17 Percentile:34.28(Geochemistry & Geophysics)

no abstracts in English

68 (Records 1-20 displayed on this page)